Atomic Layer Deposition of TiO

Additional resources and features associated with this article are available within the HTML version: • Supporting Information • Links to the 4 articles that cite this article, as of the time of this article download • Access to high resolution figures • Links to articles and content related to this article • Copyright permission to reproduce figures and/or text from this article High surface area mesoporous aerogel films were prepared on conductive glass substrates. Atomic layer deposition was employed to coat the aerogel template conformally with various thicknesses of TiO 2 with subnanometer precision. The TiO 2-coated aerogel membranes were incorporated as photoanodes in dye-sensitized solar cells. The charge diffusion length was found to increase with increasing thickness of TiO 2 leading to increasing current and efficiency. Initial devices exhibited power conversion efficiencies of up to 4.3% under 100 W m-2 light intensity. The novel fabrication technique provides a facile, oxide materials general method to prepare high surface area pseudo-one-dimensional DSSC photoanodes with promising performance.